Highly efficient polariton emission of an ultrastrongly coupled MDMO-PPV OLED

Jui Fen Chang; Guo Sian Ciou; Wei Hong Lin; Gui Sheng Zeng; Sheng Hui Chen; Po Hsiang Huang

doi:10.35848/1347-4065/ac4c25

Highly efficient polariton emission of an ultrastrongly coupled MDMO-PPV OLED

Jui Fen Chang, Guo Sian Ciou, Wei Hong Lin, Gui Sheng Zeng, Sheng Hui Chen, Po Hsiang Huang

光電科學與工程學系

研究成果: 雜誌貢獻 › 期刊論文 › 同行評審

7 引文斯高帕斯（Scopus）

摘要

We report on a highly efficient polariton emission of poly [2-methoxy-5-(3, 7-dimethyloctyloxy)-1, 4-phenylenevinylene] (MDMO-PPV) organic light-emitting diode (OLED) operating in the ultrastrong coupling regime. MDMO-PPV film with a broadband high absorbance and modest Stokes shift is shown to enable the generation of a large coupling strength and radiative pumping of the lower polariton (LP) mode. Further combining the optimized conditions of cavity design, electron injection, and emission side mirror, we demonstrate that the polariton OLED can produce a spectrally narrow and almost angle-independent emission from the LP mode, with a maximum external quantum efficiency of >0.1% and a Rabi splitting energy of >0.8 eV.

原文	???core.languages.en_GB???
文章編號	020906
期刊	Japanese Journal of Applied Physics
卷	61
發行號	2
DOIs	https://doi.org/10.35848/1347-4065/ac4c25
出版狀態	已出版 - 1 2月 2022

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10.35848/1347-4065/ac4c25

高發光效率之有機強耦合/超強耦合元件開發與偏極子物理研究
Chang, J.-F. (PI)
1/08/21 → 31/07/23
研究計畫: Research

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title = "Highly efficient polariton emission of an ultrastrongly coupled MDMO-PPV OLED",

abstract = "We report on a highly efficient polariton emission of poly [2-methoxy-5-(3, 7-dimethyloctyloxy)-1, 4-phenylenevinylene] (MDMO-PPV) organic light-emitting diode (OLED) operating in the ultrastrong coupling regime. MDMO-PPV film with a broadband high absorbance and modest Stokes shift is shown to enable the generation of a large coupling strength and radiative pumping of the lower polariton (LP) mode. Further combining the optimized conditions of cavity design, electron injection, and emission side mirror, we demonstrate that the polariton OLED can produce a spectrally narrow and almost angle-independent emission from the LP mode, with a maximum external quantum efficiency of >0.1% and a Rabi splitting energy of >0.8 eV.",

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T1 - Highly efficient polariton emission of an ultrastrongly coupled MDMO-PPV OLED

AU - Chang, Jui Fen

AU - Ciou, Guo Sian

AU - Lin, Wei Hong

AU - Zeng, Gui Sheng

AU - Chen, Sheng Hui

AU - Huang, Po Hsiang

PY - 2022/2/1

Y1 - 2022/2/1

N2 - We report on a highly efficient polariton emission of poly [2-methoxy-5-(3, 7-dimethyloctyloxy)-1, 4-phenylenevinylene] (MDMO-PPV) organic light-emitting diode (OLED) operating in the ultrastrong coupling regime. MDMO-PPV film with a broadband high absorbance and modest Stokes shift is shown to enable the generation of a large coupling strength and radiative pumping of the lower polariton (LP) mode. Further combining the optimized conditions of cavity design, electron injection, and emission side mirror, we demonstrate that the polariton OLED can produce a spectrally narrow and almost angle-independent emission from the LP mode, with a maximum external quantum efficiency of >0.1% and a Rabi splitting energy of >0.8 eV.

AB - We report on a highly efficient polariton emission of poly [2-methoxy-5-(3, 7-dimethyloctyloxy)-1, 4-phenylenevinylene] (MDMO-PPV) organic light-emitting diode (OLED) operating in the ultrastrong coupling regime. MDMO-PPV film with a broadband high absorbance and modest Stokes shift is shown to enable the generation of a large coupling strength and radiative pumping of the lower polariton (LP) mode. Further combining the optimized conditions of cavity design, electron injection, and emission side mirror, we demonstrate that the polariton OLED can produce a spectrally narrow and almost angle-independent emission from the LP mode, with a maximum external quantum efficiency of >0.1% and a Rabi splitting energy of >0.8 eV.

KW - OLED

KW - polariton

KW - ultrastrong coupling

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DO - 10.35848/1347-4065/ac4c25

M3 - 期刊論文

AN - SCOPUS:85125597601

SN - 0021-4922

VL - 61

JO - Japanese Journal of Applied Physics

JF - Japanese Journal of Applied Physics

IS - 2

M1 - 020906

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Highly efficient polariton emission of an ultrastrongly coupled MDMO-PPV OLED

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高發光效率之有機強耦合/超強耦合元件開發與偏極子物理研究

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