TY - JOUR
T1 - High Efficiency and Uniform Emission in Micropixelated Inorganic/Organic Hybrid Vertical Light-Emitting Transistors and Displays
AU - Chang, Jui Fen
AU - Huang, Guang Ru
AU - Wu, Yu Pei
AU - Chang, Chih Hao
AU - Lo, Yu Jen
AU - Yu, Jia Min
N1 - Publisher Copyright:
© 2022 American Chemical Society.
PY - 2022/12/27
Y1 - 2022/12/27
N2 - Vertical light-emitting transistors (VLETs) fabricated by integrating organic vertical transistors and organic light-emitting diodes (OLEDs) have been proposed as a prospective building block for display technologies. However, organic vertical transistors normally have non-ohmic injection and a low-mobility channel, resulting in low VLET performance compared to the pristine OLED. The difficulty of fine patterning the source electrode and organic layer in a stacked VLET geometry has also been a technical issue limiting industrial applications. This paper reports on a simple approach to realize a high-performance, miniaturized VLET by using a highly conductive, well-designed inorganic transistor. Here, we investigate the ZnO transistor configured with an insulator-encapsulated source electrode to confine the current pathway in the VLET, which can be easily fabricated and integrated with various solution-processed or vacuum-sublimed inverted OLEDs (IOLEDs). This ZnO transistor exhibits ohmic contact and a high electron mobility of >10 cm2/(V s) that enables effective electron injection and lateral transport in the VLET, forming a millimeter-scale density gradient (channel depth) for strong surface emission. Furthermore, the high mobility of ZnO facilitates the design of a simple source pattern with a large aperture ratio on the ZnO area to control the current density and distribution and thus the VLET output. From a systematic study of the source design, we show that the ZnO transistor can be optimized to achieve homogeneously high conductivity in the ON state and yield the best VLET performance with maximum emission intensity and efficiency close to those of the IOLED, while the emission can be spatially uniform and precisely defined by the ZnO pattern. Finally, we implement a micropixelated VLET-based active matrix panel to demonstrate the prospect of high-resolution display applications.
AB - Vertical light-emitting transistors (VLETs) fabricated by integrating organic vertical transistors and organic light-emitting diodes (OLEDs) have been proposed as a prospective building block for display technologies. However, organic vertical transistors normally have non-ohmic injection and a low-mobility channel, resulting in low VLET performance compared to the pristine OLED. The difficulty of fine patterning the source electrode and organic layer in a stacked VLET geometry has also been a technical issue limiting industrial applications. This paper reports on a simple approach to realize a high-performance, miniaturized VLET by using a highly conductive, well-designed inorganic transistor. Here, we investigate the ZnO transistor configured with an insulator-encapsulated source electrode to confine the current pathway in the VLET, which can be easily fabricated and integrated with various solution-processed or vacuum-sublimed inverted OLEDs (IOLEDs). This ZnO transistor exhibits ohmic contact and a high electron mobility of >10 cm2/(V s) that enables effective electron injection and lateral transport in the VLET, forming a millimeter-scale density gradient (channel depth) for strong surface emission. Furthermore, the high mobility of ZnO facilitates the design of a simple source pattern with a large aperture ratio on the ZnO area to control the current density and distribution and thus the VLET output. From a systematic study of the source design, we show that the ZnO transistor can be optimized to achieve homogeneously high conductivity in the ON state and yield the best VLET performance with maximum emission intensity and efficiency close to those of the IOLED, while the emission can be spatially uniform and precisely defined by the ZnO pattern. Finally, we implement a micropixelated VLET-based active matrix panel to demonstrate the prospect of high-resolution display applications.
KW - active matrix displays
KW - charge transport
KW - inorganic transistors
KW - organic light-emitting diodes
KW - vertical light-emitting transistors
UR - http://www.scopus.com/inward/record.url?scp=85143605558&partnerID=8YFLogxK
U2 - 10.1021/acsaelm.2c00895
DO - 10.1021/acsaelm.2c00895
M3 - 期刊論文
AN - SCOPUS:85143605558
SN - 2637-6113
VL - 4
SP - 5752
EP - 5762
JO - ACS Applied Electronic Materials
JF - ACS Applied Electronic Materials
IS - 12
ER -