Experimental study on the performance of oxidative dry reforming from simulated biogas

Ming Pin Lai, Wei Hsiang Lai, Rong Fang Horng, Chen Yu Chen, Wei Cheng Chiu, Siou Sheng Su, You Ming Chang

研究成果: 會議貢獻類型會議論文同行評審

3 引文 斯高帕斯(Scopus)

摘要

This study was to investigate the CO2 reforming under isothermal condition. The fuel conversion efficiency and hydrogen-rich gas production were enhanced via the oxidative dry reforming (ODR) from simulated biogas (50%-CH4+50%-CO2). This paper covers two subjects. The first was to investigate the CO2 conversion characteristics under various feeding molar ratios (e.g. H2/CO2 and O2/CH4 molar ratio ). In the second, the whole performance index of the reformer was investigated. The experimental results demonstrate that the CO2 reduction capacity of methane is superior to that of hydrogen. This effect is clearer under higher reaction temperatures. The ODR reaction experiment results indicate that adding appropriate amounts of oxidants can increases the methane conversion and reforming efficiency. But, the excessive oxidizes could be reduce the CO 2 conversion efficiency. Additionally, at high DR/ODR reaction temperatures, reverse water-gas shifting (RWGS) side reactions become signification, which can reduce CO2 to CO efficiently, thereby improving the CO2 conversion efficiency. Overall, the optimal methane conversion efficiency can reach 100% in ODR reaction (O2/CH 4 molar ratio=0.5). The CO2 conversion efficiency is based on DR reactions (CO2/CH4 molar ratio=1) reaching between 57% and 95%.

原文???core.languages.en_GB???
頁面225-233
頁數9
DOIs
出版狀態已出版 - 2012
事件19th World Hydrogen Energy Conference, WHEC 2012 - Toronto, ON, Canada
持續時間: 3 6月 20127 6月 2012

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???event.eventtypes.event.conference???19th World Hydrogen Energy Conference, WHEC 2012
國家/地區Canada
城市Toronto, ON
期間3/06/127/06/12

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