Charged Hole-Transporting Materials Based on Imidazolium for Defect Passivation in Inverted Perovskite Solar Cells

Yogesh S. Tingare, Meng Che Li, Sheng Hung Teng, Ja Hon Lin, Chaochin Su, Shan Jung Lin, Xin Rui Lew, Hsinhan Tsai, Dibyajyoti Ghosh, Wanyi Nie, Bao Lin Yeh, Wen Ren Li

研究成果: 雜誌貢獻期刊論文同行評審

3 引文 斯高帕斯(Scopus)

摘要

The hole-transporting material (HTM) in perovskite solar cells (PSCs) provides an ideal interface with the perovskite layer for hole collection while influencing the perovskite crystalline structure and morphology. This article presents SIM and DIM, two new dopant-free imidazolium-based HTMs with charged units accompanied by counter ions that show the potential to function as ionic HTMs and ionic liquid additives and help improve the efficiency and stability of inverted PSCs. DIM-based PSCs demonstrates exceptional performance with a high-power conversion efficiency of 19.15%, attributed to improved passivation of perovskite interface defects. Furthermore, these new imidazolium salt-based HTMs can be manufactured economically, making them a viable option for mass production and PSC commercialization.

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文章編號2300817
期刊Solar RRL
8
發行號3
DOIs
出版狀態已出版 - 2月 2024

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