The origin of plutonium in the atmosphere

S. C. Lee, H. H.S.C. Rao, Y. Sakuragi, N. Bakhtiar, F. S. Jiang, P. K. Kuroda

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

Radiochemical measurements of 239,240 Pu were carried out for a total of 288 individual rain and snow samples collected at Fayetteville (36°N, 94°W), Arkansas, during the period between February 1976 and October 1984, The results indicate that the plutonium inventory in the northern stratosphere has been decreasing during the past several years at a rate corresponding to about 1,2 years for the mean strato-spheric residence time of plutonium. However, the fallout of plutonium may not be attributable solely to the atmospheric injections of nuclear debris from the weapons tests. It appears that the recent volcanic eruptions may have played an important role in altering the stratospheric inventory of plutonium.

Original languageEnglish
Pages (from-to)283-288
Number of pages6
JournalGEOCHEMICAL JOURNAL
Volume19
Issue number5
DOIs
StatePublished - 1986

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