Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test

S. S. Shy; Y. T. Hung; Z. H. Chou; Z. L. Bong; J. J. Jhao

doi:10.1149/09101.0745ecst

Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test

S. S. Shy, Y. T. Hung, Z. H. Chou, Z. L. Bong, J. J. Jhao

Department of Mechanical Engineering

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

1 Scopus citations

Abstract

This paper reports a stability test comparison between ammonia- and syngas-fueled anode-supported cells (ASC). The planar (50 x 50 mm²) ASC is consisted of 400-µm-Ni-YSZ anode, 3-µm-YSZ electrolyte, and 12-µm-LSC-GDC cathode together with metallic frames and current collectors which are sandwiched by a pair of rib-channel flow distributors (interconnectors) with guide vanes on both anode and cathode sides to form a single-full-cell stack in a dual-chamber pressure/temperature-controlled facility. Pressurization enhances the power density noticeably for both ammonia- and syngas-fueled ASCs. Little degradation is observed for the pressurized ammonia-fueled ASC at 0.8 V at 700^oC (power density and stability increase with increasing temperature). However, the syngas-fueled ASC can only remain stable at 1 atm and at higher temperature (≥ 800^oC); after five hours stable operation, a rapid degradation is observed at 3 atm due to severe carbon deposition even at 850^oC.

Original language	English
Title of host publication	Solid Oxide Fuel Cells 16, SOFC 2019
Editors	K. Eguchi, S. C. Singhal
Publisher	Electrochemical Society Inc.
Pages	745-752
Number of pages	8
Edition	1
ISBN (Electronic)	9781607688747, 9781607688747
DOIs	https://doi.org/10.1149/09101.0745ecst
State	Published - 2019
Event	16th International Symposium on Solid Oxide Fuel Cells, SOFC 2019 - Kyoto, Japan Duration: 8 Sep 2019 → 13 Sep 2019

Publication series

Name	ECS Transactions
Number	1
Volume	91
ISSN (Print)	1938-6737
ISSN (Electronic)	1938-5862

Conference

Conference	16th International Symposium on Solid Oxide Fuel Cells, SOFC 2019
Country/Territory	Japan
City	Kyoto
Period	8/09/19 → 13/09/19

Access to Document

10.1149/09101.0745ecst

Advanced Ammonia Sofc Full Cell Manufacture, Assembly and Testing and Its Conceptual Design for Portable Power Source(2/3)
Shy, S.-Y. (PI)
1/08/18 → 31/07/19
Project: Research

Cite this

Shy, S. S., Hung, Y. T., Chou, Z. H., Bong, Z. L., & Jhao, J. J. (2019). Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test. In K. Eguchi, & S. C. Singhal (Eds.), Solid Oxide Fuel Cells 16, SOFC 2019 (1 ed., pp. 745-752). (ECS Transactions; Vol. 91, No. 1). Electrochemical Society Inc.. https://doi.org/10.1149/09101.0745ecst

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abstract = "This paper reports a stability test comparison between ammonia- and syngas-fueled anode-supported cells (ASC). The planar (50 x 50 mm2) ASC is consisted of 400-µm-Ni-YSZ anode, 3-µm-YSZ electrolyte, and 12-µm-LSC-GDC cathode together with metallic frames and current collectors which are sandwiched by a pair of rib-channel flow distributors (interconnectors) with guide vanes on both anode and cathode sides to form a single-full-cell stack in a dual-chamber pressure/temperature-controlled facility. Pressurization enhances the power density noticeably for both ammonia- and syngas-fueled ASCs. Little degradation is observed for the pressurized ammonia-fueled ASC at 0.8 V at 700oC (power density and stability increase with increasing temperature). However, the syngas-fueled ASC can only remain stable at 1 atm and at higher temperature (≥ 800oC); after five hours stable operation, a rapid degradation is observed at 3 atm due to severe carbon deposition even at 850oC.",

author = "Shy, {S. S.} and Hung, {Y. T.} and Chou, {Z. H.} and Bong, {Z. L.} and Jhao, {J. J.}",

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Shy, SS, Hung, YT, Chou, ZH, Bong, ZL & Jhao, JJ 2019, Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test. in K Eguchi & SC Singhal (eds), Solid Oxide Fuel Cells 16, SOFC 2019. 1 edn, ECS Transactions, no. 1, vol. 91, Electrochemical Society Inc., pp. 745-752, 16th International Symposium on Solid Oxide Fuel Cells, SOFC 2019, Kyoto, Japan, 8/09/19. https://doi.org/10.1149/09101.0745ecst

Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test. / Shy, S. S.; Hung, Y. T.; Chou, Z. H. et al.
Solid Oxide Fuel Cells 16, SOFC 2019. ed. / K. Eguchi; S. C. Singhal. 1. ed. Electrochemical Society Inc., 2019. p. 745-752 (ECS Transactions; Vol. 91, No. 1).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

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AU - Jhao, J. J.

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N2 - This paper reports a stability test comparison between ammonia- and syngas-fueled anode-supported cells (ASC). The planar (50 x 50 mm2) ASC is consisted of 400-µm-Ni-YSZ anode, 3-µm-YSZ electrolyte, and 12-µm-LSC-GDC cathode together with metallic frames and current collectors which are sandwiched by a pair of rib-channel flow distributors (interconnectors) with guide vanes on both anode and cathode sides to form a single-full-cell stack in a dual-chamber pressure/temperature-controlled facility. Pressurization enhances the power density noticeably for both ammonia- and syngas-fueled ASCs. Little degradation is observed for the pressurized ammonia-fueled ASC at 0.8 V at 700oC (power density and stability increase with increasing temperature). However, the syngas-fueled ASC can only remain stable at 1 atm and at higher temperature (≥ 800oC); after five hours stable operation, a rapid degradation is observed at 3 atm due to severe carbon deposition even at 850oC.

AB - This paper reports a stability test comparison between ammonia- and syngas-fueled anode-supported cells (ASC). The planar (50 x 50 mm2) ASC is consisted of 400-µm-Ni-YSZ anode, 3-µm-YSZ electrolyte, and 12-µm-LSC-GDC cathode together with metallic frames and current collectors which are sandwiched by a pair of rib-channel flow distributors (interconnectors) with guide vanes on both anode and cathode sides to form a single-full-cell stack in a dual-chamber pressure/temperature-controlled facility. Pressurization enhances the power density noticeably for both ammonia- and syngas-fueled ASCs. Little degradation is observed for the pressurized ammonia-fueled ASC at 0.8 V at 700oC (power density and stability increase with increasing temperature). However, the syngas-fueled ASC can only remain stable at 1 atm and at higher temperature (≥ 800oC); after five hours stable operation, a rapid degradation is observed at 3 atm due to severe carbon deposition even at 850oC.

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PB - Electrochemical Society Inc.

T2 - 16th International Symposium on Solid Oxide Fuel Cells, SOFC 2019

Y2 - 8 September 2019 through 13 September 2019

ER -

Pressurized ammonia and syngas planar anode-supported solid oxide fuel cells and their performance stability test

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Advanced Ammonia Sofc Full Cell Manufacture, Assembly and Testing and Its Conceptual Design for Portable Power Source(2/3)

Cite this