Effect of pore diffusion on the rate of methanation reaction in a heterogeneous catalyst

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Abstract

A theoretical analysis is presented to describe the rate data in terms of fundamental reaction steps involved in the overall methanation kinetics. A model involving reaction inhibition (by adsorbed CO) was used in combination with the physical properties of the catalysts to determine the ranges of temperature and partial pressure of CO where pore diffusion significantly influences the observed methanation rate.

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